I can + Add language via the according button but I do not see a way to remove one:
This is for v8.7.1 but the same applies for v6.6. My account is in the sonar-administrators group on both instances (but on the latter I can't even add a language.)
The documentation for Project settings doesn't mention anything about it.
There’s actually two other ways to “disable” a language:
Source: https://community.sonarsource.com/t/how-to-turn-off-analysis-for-specific-languages/21671